PM10 concs in UK section 6 6 PM10 Projections for roadside monitoring sites

The receptor modelling methods have been extended to calculate projections for 1997 of roadside PM10 concentrations for comparison with the NAQS objective and EU limit values. We have used daily measurements of PM10 at the roadside along with rural sulphate values and measurements of NOx at the roadside and at a nearby urban background monitoring site. A regression analysis has been carried out to find the coefficients A, B and R:
  1. = A.Background NOx + B.Sulphate + R.Roadside enhancement of NOx + C
Where the Roadside enhancement of NOx is defined as the measured daily mean NOx concentration at the roadside site with a background daily mean NOx concentration from a nearby background site subtracted:

roadside enhancement concentration = roadside concentration - background concentration

The regression coefficients and correlation coefficients obtained from this analysis are listed in Table 6.1.

Table 6.1 Coefficients of regression analysis of roadside sites (NO
x expressed as ppb)
  Sulphate Background NOx Roadside NOx Intercept r2
London A3 2.74 0.177 0.0423 6.43 0.74
Bury Roadside 2.64 0.138 0.0662 6.90 0.71
Camden Roadside 2.33 0.120 0.0696 11.2 0.77
Haringey Roadside 2.53 0.125 0.0776 7.90 0.80
Glasgow Kerbside 3.11 0.0689 0.1234 6.92 0.79
London Hillingdon 2.42 0.135 0.0748 5.60 0.78
Marylebone Road 3.26 0.122 0.0901 6.12 0.79
Sutton Roadside 2.40 0.110 0.0961 7.04 0.74

We have then calculated projections for 2004 and 2005 and 2009 using the business as usual scenario. We have assumed that the roadside enhancement of PM
10 consists of 50% fine exhaust emissions and 50% coarse resuspended dust. This is consistent with a comparison of the roadside enhancements of PM10, PM2.5 and NOx at Marylebone Road carried out by APEG (APEG 1998). Figure 6.1 shows that the slope of the regression line between the roadside enhancement of particle concentration and the roadside enhancement of NOx for PM10 is twice the slope for PM2.5. The exhaust emissions are asumed to reduce in line with projected urban traffic emissions and the coarse resuspended dust is assumed to remain at 1997 levels.

The resulting projections are shown in Table 6.2. All sites are projected to exceed the NAQS objective in 2005 and the EU Stage 2 2009 98th percentile. Four of the sites are projected to exceed the EU 24-hour limit value in 2004, with three other sites having concentrations close to 50
mgm-3. At Marylebone Road the projected annual mean in 2004 is higher than the annual limit value of 40 mgm-3.

Table 6.2. PM
10 projections for Roadside sites based on 1997 monitoring data (mgm-3).
NAQS London A3 Roadside Bury Roadside Camden Roadside Haringey Roadside Glasgow Kerbside London Hillingdon Marylebone Road Sutton Roadside
1997 annual mean 28 30 32 26 31 25 39 24
1997 99th percentile 68 79 91 87 81 85 99 78
1997 Days>=50 7 14 32 19 19 15 26 16
Est. An. Mean 2004 24 25 28 23 26 22 32 21
Est. An. Mean 2005 23 25 28 22 26 21 32 21
Est. An. Mean 2009 21 23 26 21 24 19 29 19
99th perc. 2005 58 66 73 70 71 70 76 60
99th perc. 2009 53 61 68 64 68 65 68 58
2005 Days>=50 1 6 17 9 10 7 14 7
2009 Days>=50 0 5 13 7 3 6 10 3
EU
1997 annual mean 36 39 42 34 40 33 51 31
1997 90th percentile 57 61 62 55 61 54 76 49
1997 98th percentile 70 80 96 81 81 77 103 74
1997 Days>=50 25 47 83 51 74 50 66 34
Est. An. Mean 2004 31 33 36 30 34 29 42 27
Est. An. Mean 2009 27 30 34 27 31 25 38 25
2004 90th percentile 48 51 54 47 52 45 65 43
2009 90th percentile 60 46 50 43 48 41 59 38
2004 98th percentile 43 69 80 66 69 65 81 65
2009 98th percentile 55 62 73 62 64 61 72 58
2004 Days>=50 12 27 46 25 36 20 37 22
2009 Days>=50 6 18 36 22 20 14 20 15


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